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Junfeng Wang, Jianhuai Ye, Qi Zhang, Jian Zhao, Yangzhou Wu, Jingyi Li, Dantong Liu, Weijun Li, Yange Zhang, Cheng Wu and 17 more
) air pollution worldwide. Observations during winter haze pollution episodes in urban China show that most of this SOA originates from fossil-fuel combustion but the chemical mechanisms involved are unclear. Here we report field observations in a Beijing winter haze event that reveal fast aqueous-phase conversion of fossil-fuel primary organic aerosol (POA) to SOA at high relative humidity. Analyses of aerosol mass spectra and elemental ratios indicate that ring-breaking oxidation of POA aromatic species, leading to functionalization as carbonyls and carboxylic acids, may serve as the dominant mechanism for this SOA formation. A POA origin for SOA could explain why SOA has been decreasing over the 2013-2018 period in response to POA emission controls even as emissions of volatile organic compounds (VOCs) have remained flat.
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Wang, J., Ye, J., Zhang, Q., Zhao, J., Wu, Y., Li, J., Liu, D., Li, W., Zhang, Y., Wu, C., Xie, C., Qin, Y., Lei, Y., Huang, X., Guo, J., Liu, P., Fu, P., Li, Y., Lee, H. C., … Jacob, D. J. (2021). Aqueous production of secondary organic aerosol from fossil-fuel emissions in winter Beijing haze. Proceedings of the National Academy of Sciences, 118(8). https://doi.org/10.1073/pnas.2022179118
Wang, Junfeng, et al. "Aqueous production of secondary organic aerosol from fossil-fuel emissions in winter Beijing haze." Proceedings of the National Academy of Sciences, vol. 118, no. 8, 2021, https://doi.org/10.1073/pnas.2022179118.
Wang, Junfeng, Jianhuai Ye, Qi Zhang, Jian Zhao, Yangzhou Wu, Jingyi Li, Dantong Liu, et al. "Aqueous production of secondary organic aerosol from fossil-fuel emissions in winter Beijing haze." Proceedings of the National Academy of Sciences 118, no. 8 (2021). https://doi.org/10.1073/pnas.2022179118.
Wang J., Ye J., Zhang Q. [и др.] Aqueous production of secondary organic aerosol from fossil-fuel emissions in winter Beijing haze // Proceedings of the National Academy of Sciences. — 2021. — Vol. 118, № 8. — URL: https://doi.org/10.1073/pnas.2022179118
@article{wang2021aqueous,
title = {{Aqueous production of secondary organic aerosol from fossil-fuel emissions in winter Beijing haze}},
author = {Junfeng Wang and Jianhuai Ye and Qi Zhang and Jian Zhao and Yangzhou Wu and Jingyi Li and Dantong Liu and Weijun Li and Yange Zhang and Cheng Wu and Conghui Xie and Yiming Qin and Yali Lei and Xiangpeng Huang and Jianping Guo and Pengfei Liu and Pingqing Fu and Yongjie Li and Hyun Chul Lee and Hyoungwoo Choi and Jie Zhang and Hong Jian Liao and Mindong Chen and Yele Sun and Xinlei Ge and Scot T. Martin and Daniel J. Jacob},
journal = {Proceedings of the National Academy of Sciences},
year = {2021},
volume = {118},
number = {8},
doi = {10.1073/pnas.2022179118},
url = {https://doi.org/10.1073/pnas.2022179118}
}TY - JOUR AU - Wang, Junfeng AU - Ye, Jianhuai AU - Zhang, Qi AU - Zhao, Jian AU - Wu, Yangzhou AU - Li, Jingyi AU - Liu, Dantong AU - Li, Weijun AU - Zhang, Yange AU - Wu, Cheng AU - Xie, Conghui AU - Qin, Yiming AU - Lei, Yali AU - Huang, Xiangpeng AU - Guo, Jianping AU - Liu, Pengfei AU - Fu, Pingqing AU - Li, Yongjie AU - Lee, Hyun Chul AU - Choi, Hyoungwoo AU - Zhang, Jie AU - Liao, Hong Jian AU - Chen, Mindong AU - Sun, Yele AU - Ge, Xinlei AU - Martin, Scot T. AU - Jacob, Daniel J. TI - Aqueous production of secondary organic aerosol from fossil-fuel emissions in winter Beijing haze JO - Proceedings of the National Academy of Sciences VL - 118 IS - 8 PY - 2021 DA - 2021/02/15 DO - 10.1073/pnas.2022179118 UR - https://doi.org/10.1073/pnas.2022179118 ER -
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