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Sungho Jeon, Taeyeong Heo, Sang-Yeon Hwang, Jim Ciston, Karen C. Bustillo, Bryan W. Reed, Jimin Ham, Sungsu Kang, Sungin Kim, Joowon Lim and 11 more
Nucleation in atomic crystallization remains poorly understood, despite advances in classical nucleation theory. The nucleation process has been described to involve a nonclassical mechanism that includes a spontaneous transition from disordered to crystalline states, but a detailed understanding of dynamics requires further investigation. In situ electron microscopy of heterogeneous nucleation of individual gold nanocrystals with millisecond temporal resolution shows that the early stage of atomic crystallization proceeds through dynamic structural fluctuations between disordered and crystalline states, rather than through a single irreversible transition. Our experimental and theoretical analyses support the idea that structural fluctuations originate from size-dependent thermodynamic stability of the two states in atomic clusters. These findings, based on dynamics in a real atomic system, reshape and improve our understanding of nucleation mechanisms in atomic crystallization.
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Jeon, S., Heo, T., Hwang, S.-Y., Ciston, J., Bustillo, K. C., Reed, B. W., Ham, J., Kang, S., Kim, S., Lim, J., Lim, K., Kim, J. S., Kang, M., Bloom, R., Hong, S., Kim, K., Zettl, A. K., Kim, W. Y., Ercius, P. A., … Lee, W. C. (2021). Reversible disorder-order transitions in atomic crystal nucleation. Science, 371(6528), 498–503. https://doi.org/10.1126/science.aaz7555
Jeon, Sungho, et al. "Reversible disorder-order transitions in atomic crystal nucleation." Science, vol. 371, no. 6528, 2021, pp. 498–503, https://doi.org/10.1126/science.aaz7555.
Jeon, Sungho, Taeyeong Heo, Sang-Yeon Hwang, Jim Ciston, Karen C. Bustillo, Bryan W. Reed, Jimin Ham, et al. "Reversible disorder-order transitions in atomic crystal nucleation." Science 371, no. 6528 (2021): 498–503. https://doi.org/10.1126/science.aaz7555.
Jeon S., Heo T., Hwang S.-Y. [и др.] Reversible disorder-order transitions in atomic crystal nucleation // Science. — 2021. — Vol. 371, № 6528. — P. 498–503. — URL: https://doi.org/10.1126/science.aaz7555
@article{jeon2021reversible,
title = {{Reversible disorder-order transitions in atomic crystal nucleation}},
author = {Sungho Jeon and Taeyeong Heo and Sang-Yeon Hwang and Jim Ciston and Karen C. Bustillo and Bryan W. Reed and Jimin Ham and Sungsu Kang and Sungin Kim and Joowon Lim and Kitaek Lim and Ji Soo Kim and Min‐Ho Kang and Ruth Bloom and Sukjoon Hong and Kwanpyo Kim and Alex K. Zettl and Woo Youn Kim and Peter A. Ercius and Jungwon Park and Won Chul Lee},
journal = {Science},
year = {2021},
volume = {371},
number = {6528},
pages = {498--503},
doi = {10.1126/science.aaz7555},
url = {https://doi.org/10.1126/science.aaz7555}
}TY - JOUR AU - Jeon, Sungho AU - Heo, Taeyeong AU - Hwang, Sang-Yeon AU - Ciston, Jim AU - Bustillo, Karen C. AU - Reed, Bryan W. AU - Ham, Jimin AU - Kang, Sungsu AU - Kim, Sungin AU - Lim, Joowon AU - Lim, Kitaek AU - Kim, Ji Soo AU - Kang, Min‐Ho AU - Bloom, Ruth AU - Hong, Sukjoon AU - Kim, Kwanpyo AU - Zettl, Alex K. AU - Kim, Woo Youn AU - Ercius, Peter A. AU - Park, Jungwon AU - Lee, Won Chul TI - Reversible disorder-order transitions in atomic crystal nucleation JO - Science VL - 371 IS - 6528 SP - 498 EP - 503 PY - 2021 DA - 2021/01/28 DO - 10.1126/science.aaz7555 UR - https://doi.org/10.1126/science.aaz7555 ER -
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