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Yanfei Xu, Xiangyang Li, Junhu Gao, Jie Wang, Guangyuan Ma, Xiaodong Wen, Yong Ping Yang, Yongwang Li, Mingyue Ding
Keeping water away Syngas, a mixture of carbon monoxide (CO) and hydrogen, allows nonpetroleum resources such as biomass and natural gas to be converted to chemical products through Fischer-Tropsch synthesis. However, for the production of olefins, a key feedstock for other chemicals, about 50% of the CO is transformed to carbon dioxide and methane. Xu et al. decreased the selectivity for these undesired by-products to under 25% by modifying their catalyst, nanoparticles of iron doped with manganese and coated with a silica, with methyl groups (see the Perspective by Xie). This hydrophobic surface shortens the retention time of water on the catalyst surface to avoid the unwanted side reactions, and also suppresses oxidation of the metal carbide catalyst that forms under reaction conditions. Science , this issue p. 610 ; see also p. 577
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Xu, Y., Li, X., Gao, J., Wang, J., Ma, G., Wen, X., Yang, Y. P., Li, Y., & Ding, M. (2021). A hydrophobic FeMn@Si catalyst increases olefins from syngas by suppressing C1 by-products. Science, 371(6529), 610–613. https://doi.org/10.1126/science.abb3649
Xu, Yanfei, et al. "A hydrophobic FeMn@Si catalyst increases olefins from syngas by suppressing C1 by-products." Science, vol. 371, no. 6529, 2021, pp. 610–613, https://doi.org/10.1126/science.abb3649.
Xu, Yanfei, Xiangyang Li, Junhu Gao, Jie Wang, Guangyuan Ma, Xiaodong Wen, Yong Ping Yang, Yongwang Li, and Mingyue Ding. "A hydrophobic FeMn@Si catalyst increases olefins from syngas by suppressing C1 by-products." Science 371, no. 6529 (2021): 610–613. https://doi.org/10.1126/science.abb3649.
Xu Y., Li X., Gao J. [и др.] A hydrophobic FeMn@Si catalyst increases olefins from syngas by suppressing C1 by-products // Science. — 2021. — Vol. 371, № 6529. — P. 610–613. — URL: https://doi.org/10.1126/science.abb3649
@article{xu2021hydrophobic,
title = {{A hydrophobic FeMn@Si catalyst increases olefins from syngas by suppressing C1 by-products}},
author = {Yanfei Xu and Xiangyang Li and Junhu Gao and Jie Wang and Guangyuan Ma and Xiaodong Wen and Yong Ping Yang and Yongwang Li and Mingyue Ding},
journal = {Science},
year = {2021},
volume = {371},
number = {6529},
pages = {610--613},
doi = {10.1126/science.abb3649},
url = {https://doi.org/10.1126/science.abb3649}
}TY - JOUR AU - Xu, Yanfei AU - Li, Xiangyang AU - Gao, Junhu AU - Wang, Jie AU - Ma, Guangyuan AU - Wen, Xiaodong AU - Yang, Yong Ping AU - Li, Yongwang AU - Ding, Mingyue TI - A hydrophobic FeMn@Si catalyst increases olefins from syngas by suppressing C1 by-products JO - Science VL - 371 IS - 6529 SP - 610 EP - 613 PY - 2021 DA - 2021/02/04 DO - 10.1126/science.abb3649 UR - https://doi.org/10.1126/science.abb3649 ER -
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