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Young‐Hoon Kim, Yaxin Zhai, Haipeng Lu, Xin Pan, Chuanxiao Xiao, E. Ashley Gaulding, Steven P. Harvey, Joseph J. Berry, Zeev Valy Vardeny, Joseph M. Luther, Matthew C. Beard
In traditional optoelectronic approaches, control over spin, charge, and light requires the use of both electrical and magnetic fields. In a spin-polarized light-emitting diode (spin-LED), charges are injected, and circularly polarized light is emitted from spin-polarized carrier pairs. Typically, the injection of carriers occurs with the application of an electric field, whereas spin polarization can be achieved using an applied magnetic field or polarized ferromagnetic contacts. We used chiral-induced spin selectivity (CISS) to produce spin-polarized carriers and demonstrate a spin-LED that operates at room temperature without magnetic fields or ferromagnetic contacts. The CISS layer consists of oriented, self-assembled small chiral molecules within a layered organic-inorganic metal-halide hybrid semiconductor framework. The spin-LED achieves ±2.6% circularly polarized electroluminescence at room temperature.
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Kim, Y., Zhai, Y., Lu, H., Pan, X., Xiao, C., Gaulding, E. A., Harvey, S. P., Berry, J. J., Vardeny, Z. V., Luther, J. M., & Beard, M. C. (2021). Chiral-induced spin selectivity enables a room-temperature spin light-emitting diode. Science, 371(6534), 1129–1133. https://doi.org/10.1126/science.abf5291
Kim, Young‐Hoon, et al. "Chiral-induced spin selectivity enables a room-temperature spin light-emitting diode." Science, vol. 371, no. 6534, 2021, pp. 1129–1133, https://doi.org/10.1126/science.abf5291.
Kim, Young‐Hoon, Yaxin Zhai, Haipeng Lu, Xin Pan, Chuanxiao Xiao, E. Ashley Gaulding, Steven P. Harvey, et al. "Chiral-induced spin selectivity enables a room-temperature spin light-emitting diode." Science 371, no. 6534 (2021): 1129–1133. https://doi.org/10.1126/science.abf5291.
Kim Y., Zhai Y., Lu H. [и др.] Chiral-induced spin selectivity enables a room-temperature spin light-emitting diode // Science. — 2021. — Vol. 371, № 6534. — P. 1129–1133. — URL: https://doi.org/10.1126/science.abf5291
@article{kim2021chiralinduced,
title = {{Chiral-induced spin selectivity enables a room-temperature spin light-emitting diode}},
author = {Young‐Hoon Kim and Yaxin Zhai and Haipeng Lu and Xin Pan and Chuanxiao Xiao and E. Ashley Gaulding and Steven P. Harvey and Joseph J. Berry and Zeev Valy Vardeny and Joseph M. Luther and Matthew C. Beard},
journal = {Science},
year = {2021},
volume = {371},
number = {6534},
pages = {1129--1133},
doi = {10.1126/science.abf5291},
url = {https://doi.org/10.1126/science.abf5291}
}TY - JOUR AU - Kim, Young‐Hoon AU - Zhai, Yaxin AU - Lu, Haipeng AU - Pan, Xin AU - Xiao, Chuanxiao AU - Gaulding, E. Ashley AU - Harvey, Steven P. AU - Berry, Joseph J. AU - Vardeny, Zeev Valy AU - Luther, Joseph M. AU - Beard, Matthew C. TI - Chiral-induced spin selectivity enables a room-temperature spin light-emitting diode JO - Science VL - 371 IS - 6534 SP - 1129 EP - 1133 PY - 2021 DA - 2021/03/11 DO - 10.1126/science.abf5291 UR - https://doi.org/10.1126/science.abf5291 ER -
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