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Bryan H. R. Suryanto, Karolina Matuszek, Jaecheol Choi, Rebecca Y. Hodgetts, Hoang‐Long Du, Jacinta M. Bakker, Colin S. M. Kang, Pavel V. Cherepanov, Alexandr N. Simonov, Douglas Robert MacFarlane
Shuttling protons in ammonia synthesis An electrochemical route to ammonia could substantially lower the greenhouse gas emissions associated with the current thermal Haber-Bosch process. One relatively promising option under study involves reductive formation of lithium nitride, which can be protonated to ammonia. However, the ethanol used to date as a local proton source in these studies may degrade under the reaction conditions. Suryanto et al. report the use of a tetraalkyl phosphonium salt in place of ethanol (see the Perspective by Westhead et al. ). This cation can stably undergo deprotonation–reprotonation cycles and, as an added benefit, it enhances the ionic conductivity of the medium. Science , abg2371, this issue p. 1187 ; see also abi8329, p. 1149
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Suryanto, B. H. R., Matuszek, K., Choi, J., Hodgetts, R. Y., Du, H., Bakker, J. M., Kang, C. S. M., Cherepanov, P. V., Simonov, A. N., & MacFarlane, D. R. (2021). Nitrogen reduction to ammonia at high efficiency and rates based on a phosphonium proton shuttle. Science, 372(6547), 1187–1191. https://doi.org/10.1126/science.abg2371
Suryanto, Bryan H. R., et al. "Nitrogen reduction to ammonia at high efficiency and rates based on a phosphonium proton shuttle." Science, vol. 372, no. 6547, 2021, pp. 1187–1191, https://doi.org/10.1126/science.abg2371.
Suryanto, Bryan H. R., Karolina Matuszek, Jaecheol Choi, Rebecca Y. Hodgetts, Hoang‐Long Du, Jacinta M. Bakker, Colin S. M. Kang, Pavel V. Cherepanov, Alexandr N. Simonov, and Douglas Robert MacFarlane. "Nitrogen reduction to ammonia at high efficiency and rates based on a phosphonium proton shuttle." Science 372, no. 6547 (2021): 1187–1191. https://doi.org/10.1126/science.abg2371.
Suryanto B. H. R., Matuszek K., Choi J. [и др.] Nitrogen reduction to ammonia at high efficiency and rates based on a phosphonium proton shuttle // Science. — 2021. — Vol. 372, № 6547. — P. 1187–1191. — URL: https://doi.org/10.1126/science.abg2371
@article{suryanto2021nitrogen,
title = {{Nitrogen reduction to ammonia at high efficiency and rates based on a phosphonium proton shuttle}},
author = {Bryan H. R. Suryanto and Karolina Matuszek and Jaecheol Choi and Rebecca Y. Hodgetts and Hoang‐Long Du and Jacinta M. Bakker and Colin S. M. Kang and Pavel V. Cherepanov and Alexandr N. Simonov and Douglas Robert MacFarlane},
journal = {Science},
year = {2021},
volume = {372},
number = {6547},
pages = {1187--1191},
doi = {10.1126/science.abg2371},
url = {https://doi.org/10.1126/science.abg2371}
}TY - JOUR AU - Suryanto, Bryan H. R. AU - Matuszek, Karolina AU - Choi, Jaecheol AU - Hodgetts, Rebecca Y. AU - Du, Hoang‐Long AU - Bakker, Jacinta M. AU - Kang, Colin S. M. AU - Cherepanov, Pavel V. AU - Simonov, Alexandr N. AU - MacFarlane, Douglas Robert TI - Nitrogen reduction to ammonia at high efficiency and rates based on a phosphonium proton shuttle JO - Science VL - 372 IS - 6547 SP - 1187 EP - 1191 PY - 2021 DA - 2021/06/10 DO - 10.1126/science.abg2371 UR - https://doi.org/10.1126/science.abg2371 ER -
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