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Ali Hussain Motagamwala, Rawan Almallahi, James Wortman, Valentina Omoze Igenegbai, Suljo Linic
Hitting the limits on propene synthesis The greater abundance of propane from shale gas has spurred efforts to use it as a propylene feedstock. Direct dehydrogenation catalysts consisting of platinum–tin alloy nanoparticles supported on alumina often must run with hydrogen dilution to avoid carbon buildup and excess tin to avoid alloy segregation. Motagamwala et al. report that platinum–tin nanoparticles interact more weakly with a silica support and the metals thus do not segregate. The use of undiluted reactants allowed the reaction to run near the thermodynamically limit of about 67% conversion with a selectivity to propylene of more than 99%. This catalyst also does not build up carbon and could run up to 30 hours without deactivation. Science , abg7894, this issue p. 217
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Motagamwala, A. H., Almallahi, R., Wortman, J., Igenegbai, V. O., & Linic, S. (2021). Stable and selective catalysts for propane dehydrogenation operating at thermodynamic limit. Science, 373(6551), 217–222. https://doi.org/10.1126/science.abg7894
Motagamwala, Ali Hussain, et al. "Stable and selective catalysts for propane dehydrogenation operating at thermodynamic limit." Science, vol. 373, no. 6551, 2021, pp. 217–222, https://doi.org/10.1126/science.abg7894.
Motagamwala, Ali Hussain, Rawan Almallahi, James Wortman, Valentina Omoze Igenegbai, and Suljo Linic. "Stable and selective catalysts for propane dehydrogenation operating at thermodynamic limit." Science 373, no. 6551 (2021): 217–222. https://doi.org/10.1126/science.abg7894.
Motagamwala A. H., Almallahi R., Wortman J. [и др.] Stable and selective catalysts for propane dehydrogenation operating at thermodynamic limit // Science. — 2021. — Vol. 373, № 6551. — P. 217–222. — URL: https://doi.org/10.1126/science.abg7894
@article{motagamwala2021stable,
title = {{Stable and selective catalysts for propane dehydrogenation operating at thermodynamic limit}},
author = {Ali Hussain Motagamwala and Rawan Almallahi and James Wortman and Valentina Omoze Igenegbai and Suljo Linic},
journal = {Science},
year = {2021},
volume = {373},
number = {6551},
pages = {217--222},
doi = {10.1126/science.abg7894},
url = {https://doi.org/10.1126/science.abg7894}
}TY - JOUR AU - Motagamwala, Ali Hussain AU - Almallahi, Rawan AU - Wortman, James AU - Igenegbai, Valentina Omoze AU - Linic, Suljo TI - Stable and selective catalysts for propane dehydrogenation operating at thermodynamic limit JO - Science VL - 373 IS - 6551 SP - 217 EP - 222 PY - 2021 DA - 2021/07/09 DO - 10.1126/science.abg7894 UR - https://doi.org/10.1126/science.abg7894 ER -
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