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Minjin Kim, Jaeki Jeong, Haizhou Lu, Tae Kyung Lee, Felix T. Eickemeyer, Yuhang Liu, In Woo Choi, Seung Ju Choi, Yimhyun Jo, Hak-Beom Kim and 11 more
Improvements to perovskite solar cells (PSCs) have focused on increasing their power conversion efficiency (PCE) and operational stability and maintaining high performance upon scale-up to module sizes. We report that replacing the commonly used mesoporous–titanium dioxide electron transport layer (ETL) with a thin layer of polyacrylic acid–stabilized tin(IV) oxide quantum dots (paa-QD-SnO 2 ) on the compact–titanium dioxide enhanced light capture and largely suppressed nonradiative recombination at the ETL–perovskite interface. The use of paa-QD-SnO 2 as electron-selective contact enabled PSCs (0.08 square centimeters) with a PCE of 25.7% (certified 25.4%) and high operational stability and facilitated the scale-up of the PSCs to larger areas. PCEs of 23.3, 21.7, and 20.6% were achieved for PSCs with active areas of 1, 20, and 64 square centimeters, respectively.
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Kim, M., Jeong, J., Lu, H., Lee, T. K., Eickemeyer, F. T., Liu, Y., Choi, I. W., Choi, S. J., Jo, Y., Kim, H.-B., Mo, S.-I., Kim, Y.-K., Lee, H., An, N. G., Cho, S., Tress, W. R., Zakeeruddin, S. M., Hagfeldt, A., Kim, J. Y., … Kim, D. S. (2022). Conformal quantum dot–SnO 2 layers as electron transporters for efficient perovskite solar cells. Science, 375(6578), 302–306. https://doi.org/10.1126/science.abh1885
Kim, Minjin, et al. "Conformal quantum dot–SnO 2 layers as electron transporters for efficient perovskite solar cells." Science, vol. 375, no. 6578, 2022, pp. 302–306, https://doi.org/10.1126/science.abh1885.
Kim, Minjin, Jaeki Jeong, Haizhou Lu, Tae Kyung Lee, Felix T. Eickemeyer, Yuhang Liu, In Woo Choi, et al. "Conformal quantum dot–SnO 2 layers as electron transporters for efficient perovskite solar cells." Science 375, no. 6578 (2022): 302–306. https://doi.org/10.1126/science.abh1885.
Kim M., Jeong J., Lu H. [и др.] Conformal quantum dot–SnO 2 layers as electron transporters for efficient perovskite solar cells // Science. — 2022. — Vol. 375, № 6578. — P. 302–306. — URL: https://doi.org/10.1126/science.abh1885
@article{kim2022conformal,
title = {{Conformal quantum dot–SnO 2 layers as electron transporters for efficient perovskite solar cells}},
author = {Minjin Kim and Jaeki Jeong and Haizhou Lu and Tae Kyung Lee and Felix T. Eickemeyer and Yuhang Liu and In Woo Choi and Seung Ju Choi and Yimhyun Jo and Hak-Beom Kim and Sung-In Mo and Young-Ki Kim and Heunjeong Lee and Na Gyeong An and Shinuk Cho and Wolfgang R. Tress and Shaik M. Zakeeruddin and Anders Hagfeldt and Jin Young Kim and Michaël Grätzel and Dong Suk Kim},
journal = {Science},
year = {2022},
volume = {375},
number = {6578},
pages = {302--306},
doi = {10.1126/science.abh1885},
url = {https://doi.org/10.1126/science.abh1885}
}TY - JOUR AU - Kim, Minjin AU - Jeong, Jaeki AU - Lu, Haizhou AU - Lee, Tae Kyung AU - Eickemeyer, Felix T. AU - Liu, Yuhang AU - Choi, In Woo AU - Choi, Seung Ju AU - Jo, Yimhyun AU - Kim, Hak-Beom AU - Mo, Sung-In AU - Kim, Young-Ki AU - Lee, Heunjeong AU - An, Na Gyeong AU - Cho, Shinuk AU - Tress, Wolfgang R. AU - Zakeeruddin, Shaik M. AU - Hagfeldt, Anders AU - Kim, Jin Young AU - Grätzel, Michaël AU - Kim, Dong Suk TI - Conformal quantum dot–SnO 2 layers as electron transporters for efficient perovskite solar cells JO - Science VL - 375 IS - 6578 SP - 302 EP - 306 PY - 2022 DA - 2022/01/20 DO - 10.1126/science.abh1885 UR - https://doi.org/10.1126/science.abh1885 ER -
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