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Shangshang Chen, Xuezeng Dai, Shuang Xu, Haoyang Jiao, Liang Zhao, Jinsong Huang
The interfaces of perovskite solar cells (PSCs) are important in determining their efficiency and stability, but the morphology and stability of imbedded perovskite-substrate interfaces have received less attention than have top interfaces. We found that dimethyl sulfoxide (DMSO), which is a liquid additive broadly applied to enhance perovskite film morphology, was trapped during film formation and led to voids at perovskite-substrate interfaces that accelerated the film degradation under illumination. Partial replacement of DMSO with solid-state carbohydrazide reduces interfacial voids. A maximum stabilized power conversion efficiency (PCE) of 23.6% was realized for blade-coated p-type/intrinsic/n-type (p-i-n) structure PSCs with no efficiency loss after 550-hour operational stability tests at 60°C. The perovskite mini-modules showed certified PCEs of 19.3 and 19.2%, with aperture areas of 18.1 and 50.0 square centimeters, respectively.
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Chen, S., Dai, X., Xu, S., Jiao, H., Zhao, L., & Huang, J. (2021). Stabilizing perovskite-substrate interfaces for high-performance perovskite modules. Science, 373(6557), 902–907. https://doi.org/10.1126/science.abi6323
Chen, Shangshang, et al. "Stabilizing perovskite-substrate interfaces for high-performance perovskite modules." Science, vol. 373, no. 6557, 2021, pp. 902–907, https://doi.org/10.1126/science.abi6323.
Chen, Shangshang, Xuezeng Dai, Shuang Xu, Haoyang Jiao, Liang Zhao, and Jinsong Huang. "Stabilizing perovskite-substrate interfaces for high-performance perovskite modules." Science 373, no. 6557 (2021): 902–907. https://doi.org/10.1126/science.abi6323.
Chen S., Dai X., Xu S. [и др.] Stabilizing perovskite-substrate interfaces for high-performance perovskite modules // Science. — 2021. — Vol. 373, № 6557. — P. 902–907. — URL: https://doi.org/10.1126/science.abi6323
@article{chen2021stabilizing,
title = {{Stabilizing perovskite-substrate interfaces for high-performance perovskite modules}},
author = {Shangshang Chen and Xuezeng Dai and Shuang Xu and Haoyang Jiao and Liang Zhao and Jinsong Huang},
journal = {Science},
year = {2021},
volume = {373},
number = {6557},
pages = {902--907},
doi = {10.1126/science.abi6323},
url = {https://doi.org/10.1126/science.abi6323}
}TY - JOUR AU - Chen, Shangshang AU - Dai, Xuezeng AU - Xu, Shuang AU - Jiao, Haoyang AU - Zhao, Liang AU - Huang, Jinsong TI - Stabilizing perovskite-substrate interfaces for high-performance perovskite modules JO - Science VL - 373 IS - 6557 SP - 902 EP - 907 PY - 2021 DA - 2021/08/19 DO - 10.1126/science.abi6323 UR - https://doi.org/10.1126/science.abi6323 ER -
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