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Cheng-Long Yang, Lina Wang, Peng Yin, Jieyuan Liu, Ming‐Xi Chen, Qiangqiang Yan, Zheng-Shu Wang, Shi‐Long Xu, Shengqi Chu, Chunhua Cui and 5 more
Atomically ordered intermetallic nanoparticles are promising for catalytic applications but are difficult to produce because the high-temperature annealing required for atom ordering inevitably accelerates metal sintering that leads to larger crystallites. We prepared platinum intermetallics with an average particle size of <5 nanometers on porous sulfur-doped carbon supports, on which the strong interaction between platinum and sulfur suppresses metal sintering up to 1000°C. We synthesized intermetallic libraries of small nanoparticles consisting of 46 combinations of platinum with 16 other metal elements and used them to study the dependence of electrocatalytic oxygen-reduction reaction activity on alloy composition and platinum skin strain. The intermetallic libraries are highly mass efficient in proton-exchange-membrane fuel cells and could achieve high activities of 1.3 to 1.8 amperes per milligram of platinum at 0.9 volts.
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Yang, C.-L., Wang, L., Yin, P., Liu, J., Chen, M., Yan, Q., Wang, Z.-S., Xu, S., Chu, S., Cui, C., Ju, H., Zhu, J., Lin, Y., Shui, J., & Liang, H. (2021). Sulfur-anchoring synthesis of platinum intermetallic nanoparticle catalysts for fuel cells. Science, 374(6566), 459–464. https://doi.org/10.1126/science.abj9980
Yang, Cheng-Long, et al. "Sulfur-anchoring synthesis of platinum intermetallic nanoparticle catalysts for fuel cells." Science, vol. 374, no. 6566, 2021, pp. 459–464, https://doi.org/10.1126/science.abj9980.
Yang, Cheng-Long, Lina Wang, Peng Yin, Jieyuan Liu, Ming‐Xi Chen, Qiangqiang Yan, Zheng-Shu Wang, et al. "Sulfur-anchoring synthesis of platinum intermetallic nanoparticle catalysts for fuel cells." Science 374, no. 6566 (2021): 459–464. https://doi.org/10.1126/science.abj9980.
Yang C.-L., Wang L., Yin P. [и др.] Sulfur-anchoring synthesis of platinum intermetallic nanoparticle catalysts for fuel cells // Science. — 2021. — Vol. 374, № 6566. — P. 459–464. — URL: https://doi.org/10.1126/science.abj9980
@article{yang2021sulfuranchoring,
title = {{Sulfur-anchoring synthesis of platinum intermetallic nanoparticle catalysts for fuel cells}},
author = {Cheng-Long Yang and Lina Wang and Peng Yin and Jieyuan Liu and Ming‐Xi Chen and Qiangqiang Yan and Zheng-Shu Wang and Shi‐Long Xu and Shengqi Chu and Chunhua Cui and Huanxin Ju and Junfa Zhu and Yue Lin and Jianglan Shui and Hai‐Wei Liang},
journal = {Science},
year = {2021},
volume = {374},
number = {6566},
pages = {459--464},
doi = {10.1126/science.abj9980},
url = {https://doi.org/10.1126/science.abj9980}
}TY - JOUR AU - Yang, Cheng-Long AU - Wang, Lina AU - Yin, Peng AU - Liu, Jieyuan AU - Chen, Ming‐Xi AU - Yan, Qiangqiang AU - Wang, Zheng-Shu AU - Xu, Shi‐Long AU - Chu, Shengqi AU - Cui, Chunhua AU - Ju, Huanxin AU - Zhu, Junfa AU - Lin, Yue AU - Shui, Jianglan AU - Liang, Hai‐Wei TI - Sulfur-anchoring synthesis of platinum intermetallic nanoparticle catalysts for fuel cells JO - Science VL - 374 IS - 6566 SP - 459 EP - 464 PY - 2021 DA - 2021/10/21 DO - 10.1126/science.abj9980 UR - https://doi.org/10.1126/science.abj9980 ER -
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