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Yujing Liu, Xinyong Tao, Yao Wang, Chi Jiang, Cong Ma, Ouwei Sheng, Gongxun Lu, Xiong Wen Lou
High–energy density lithium (Li) metal batteries (LMBs) are promising for energy storage applications but suffer from uncontrollable electrolyte degradation and the consequently formed unstable solid-electrolyte interphase (SEI). In this study, we designed self-assembled monolayers (SAMs) with high-density and long-range–ordered polar carboxyl groups linked to an aluminum oxide–coated separator to provide strong dipole moments, thus offering excess electrons to accelerate the degradation dynamics of carbon-fluorine bond cleavage in Li bis(trifluoromethanesulfonyl)imide. Hence, an SEI with enriched lithium fluoride (LiF) nanocrystals is generated, facilitating rapid Li + transfer and suppressing dendritic Li growth. In particular, the SAMs endow the full cells with substantially enhanced cyclability under high cathode loading, limited Li excess, and lean electrolyte conditions. As such, our work extends the long-established SAMs technology into a platform to control electrolyte degradation and SEI formation toward LMBs with ultralong life spans.
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Liu, Y., Tao, X., Wang, Y., Jiang, C., Ma, C., Sheng, O., Lu, G., & Lou, X. W. (2022). Self-assembled monolayers direct a LiF-rich interphase toward long-life lithium metal batteries. Science, 375(6582), 739–745. https://doi.org/10.1126/science.abn1818
Liu, Yujing, et al. "Self-assembled monolayers direct a LiF-rich interphase toward long-life lithium metal batteries." Science, vol. 375, no. 6582, 2022, pp. 739–745, https://doi.org/10.1126/science.abn1818.
Liu, Yujing, Xinyong Tao, Yao Wang, Chi Jiang, Cong Ma, Ouwei Sheng, Gongxun Lu, and Xiong Wen Lou. "Self-assembled monolayers direct a LiF-rich interphase toward long-life lithium metal batteries." Science 375, no. 6582 (2022): 739–745. https://doi.org/10.1126/science.abn1818.
Liu Y., Tao X., Wang Y. [и др.] Self-assembled monolayers direct a LiF-rich interphase toward long-life lithium metal batteries // Science. — 2022. — Vol. 375, № 6582. — P. 739–745. — URL: https://doi.org/10.1126/science.abn1818
@article{liu2022selfassembled,
title = {{Self-assembled monolayers direct a LiF-rich interphase toward long-life lithium metal batteries}},
author = {Yujing Liu and Xinyong Tao and Yao Wang and Chi Jiang and Cong Ma and Ouwei Sheng and Gongxun Lu and Xiong Wen Lou},
journal = {Science},
year = {2022},
volume = {375},
number = {6582},
pages = {739--745},
doi = {10.1126/science.abn1818},
url = {https://doi.org/10.1126/science.abn1818}
}TY - JOUR AU - Liu, Yujing AU - Tao, Xinyong AU - Wang, Yao AU - Jiang, Chi AU - Ma, Cong AU - Sheng, Ouwei AU - Lu, Gongxun AU - Lou, Xiong Wen TI - Self-assembled monolayers direct a LiF-rich interphase toward long-life lithium metal batteries JO - Science VL - 375 IS - 6582 SP - 739 EP - 745 PY - 2022 DA - 2022/02/17 DO - 10.1126/science.abn1818 UR - https://doi.org/10.1126/science.abn1818 ER -
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