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Yigao Yuan, Linan Zhou, Hossein Robatjazi, Junwei Lucas Bao, Jingyi Zhou, Aaron Bayles, Lin Yuan, Minghe Lou, Minhan Lou, Suman Khatiwada and 3 more
Catalysts based on platinum group metals have been a major focus of the chemical industry for decades. We show that plasmonic photocatalysis can transform a thermally unreactive, earth-abundant transition metal into a catalytically active site under illumination. Fe active sites in a Cu-Fe antenna-reactor complex achieve efficiencies very similar to Ru for the photocatalytic decomposition of ammonia under ultrafast pulsed illumination. When illuminated with light-emitting diodes rather than lasers, the photocatalytic efficiencies remain comparable, even when the scale of reaction increases by nearly three orders of magnitude. This result demonstrates the potential for highly efficient, electrically driven production of hydrogen from an ammonia carrier with earth-abundant transition metals.
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Yuan, Y., Zhou, L., Robatjazi, H., Bao, J. L., Zhou, J., Bayles, A., Yuan, L., Lou, M., Lou, M., Khatiwada, S., Carter, E. A., Nordlander, P. J., & Halas, N. J. (2022). Earth-abundant photocatalyst for H 2 generation from NH 3 with light-emitting diode illumination. Science, 378(6622), 889–893. https://doi.org/10.1126/science.abn5636
Yuan, Yigao, et al. "Earth-abundant photocatalyst for H 2 generation from NH 3 with light-emitting diode illumination." Science, vol. 378, no. 6622, 2022, pp. 889–893, https://doi.org/10.1126/science.abn5636.
Yuan, Yigao, Linan Zhou, Hossein Robatjazi, Junwei Lucas Bao, Jingyi Zhou, Aaron Bayles, Lin Yuan, et al. "Earth-abundant photocatalyst for H 2 generation from NH 3 with light-emitting diode illumination." Science 378, no. 6622 (2022): 889–893. https://doi.org/10.1126/science.abn5636.
Yuan Y., Zhou L., Robatjazi H. [и др.] Earth-abundant photocatalyst for H 2 generation from NH 3 with light-emitting diode illumination // Science. — 2022. — Vol. 378, № 6622. — P. 889–893. — URL: https://doi.org/10.1126/science.abn5636
@article{yuan2022earthabundant,
title = {{Earth-abundant photocatalyst for H 2 generation from NH 3 with light-emitting diode illumination}},
author = {Yigao Yuan and Linan Zhou and Hossein Robatjazi and Junwei Lucas Bao and Jingyi Zhou and Aaron Bayles and Lin Yuan and Minghe Lou and Minhan Lou and Suman Khatiwada and Emily A. Carter and Peter J. Nordlander and Naomi J. Halas},
journal = {Science},
year = {2022},
volume = {378},
number = {6622},
pages = {889--893},
doi = {10.1126/science.abn5636},
url = {https://doi.org/10.1126/science.abn5636}
}TY - JOUR AU - Yuan, Yigao AU - Zhou, Linan AU - Robatjazi, Hossein AU - Bao, Junwei Lucas AU - Zhou, Jingyi AU - Bayles, Aaron AU - Yuan, Lin AU - Lou, Minghe AU - Lou, Minhan AU - Khatiwada, Suman AU - Carter, Emily A. AU - Nordlander, Peter J. AU - Halas, Naomi J. TI - Earth-abundant photocatalyst for H 2 generation from NH 3 with light-emitting diode illumination JO - Science VL - 378 IS - 6622 SP - 889 EP - 893 PY - 2022 DA - 2022/11/24 DO - 10.1126/science.abn5636 UR - https://doi.org/10.1126/science.abn5636 ER -
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