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Yang Zhao, Fei Ma, Zihan Qu, Shiqi Yu, Tao Shen, Hui‐Xiong Deng, Xinbo Chu, Xinxin Peng, Yongbo Yuan, Xingwang Zhang, Jingbi You
In halide perovskite solar cells the formation of secondary-phase excess lead iodide (PbI 2 ) has some positive effects on power conversion efficiency (PCE) but can be detrimental to device stability and lead to large hysteresis effects in voltage sweeps. We converted PbI 2 into an inactive (PbI 2 ) 2 RbCl compound by RbCl doping, which effectively stabilizes the perovskite phase. We obtained a certified PCE of 25.6% for FAPbI 3 (FA, formamidinium) perovskite solar cells on the basis of this strategy. Devices retained 96% of their original PCE values after 1000 hours of shelf storage and 80% after 500 hours of thermal stability testing at 85°C.
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Zhao, Y., Ma, F., Qu, Z., Yu, S., Shen, T., Deng, H., Chu, X., Peng, X., Yuan, Y., Zhang, X., & You, J. (2022). Inactive (PbI 2 ) 2 RbCl stabilizes perovskite films for efficient solar cells. Science, 377(6605), 531–534. https://doi.org/10.1126/science.abp8873
Zhao, Yang, et al. "Inactive (PbI 2 ) 2 RbCl stabilizes perovskite films for efficient solar cells." Science, vol. 377, no. 6605, 2022, pp. 531–534, https://doi.org/10.1126/science.abp8873.
Zhao, Yang, Fei Ma, Zihan Qu, Shiqi Yu, Tao Shen, Hui‐Xiong Deng, Xinbo Chu, et al. "Inactive (PbI 2 ) 2 RbCl stabilizes perovskite films for efficient solar cells." Science 377, no. 6605 (2022): 531–534. https://doi.org/10.1126/science.abp8873.
Zhao Y., Ma F., Qu Z. [и др.] Inactive (PbI 2 ) 2 RbCl stabilizes perovskite films for efficient solar cells // Science. — 2022. — Vol. 377, № 6605. — P. 531–534. — URL: https://doi.org/10.1126/science.abp8873
@article{zhao2022inactive,
title = {{Inactive (PbI 2 ) 2 RbCl stabilizes perovskite films for efficient solar cells}},
author = {Yang Zhao and Fei Ma and Zihan Qu and Shiqi Yu and Tao Shen and Hui‐Xiong Deng and Xinbo Chu and Xinxin Peng and Yongbo Yuan and Xingwang Zhang and Jingbi You},
journal = {Science},
year = {2022},
volume = {377},
number = {6605},
pages = {531--534},
doi = {10.1126/science.abp8873},
url = {https://doi.org/10.1126/science.abp8873}
}TY - JOUR AU - Zhao, Yang AU - Ma, Fei AU - Qu, Zihan AU - Yu, Shiqi AU - Shen, Tao AU - Deng, Hui‐Xiong AU - Chu, Xinbo AU - Peng, Xinxin AU - Yuan, Yongbo AU - Zhang, Xingwang AU - You, Jingbi TI - Inactive (PbI 2 ) 2 RbCl stabilizes perovskite films for efficient solar cells JO - Science VL - 377 IS - 6605 SP - 531 EP - 534 PY - 2022 DA - 2022/07/28 DO - 10.1126/science.abp8873 UR - https://doi.org/10.1126/science.abp8873 ER -
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