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Binbin Jiang, Wu Wang, Shixuan Liu, Yan Wang, Chaofan Wang, Yani Chen, Lin Hua Xie, Mingyuan Huang, Jiaqing He
The high-entropy concept provides extended, optimized space of a composition, resulting in unusual transport phenomena and excellent thermoelectric performance. By tuning electron and phonon localization, we enhanced the figure-of-merit value to 2.7 at 750 kelvin in germanium telluride-based high-entropy materials and realized a high experimental conversion efficiency of 13.3% at a temperature difference of 506 kelvin with the fabricated segmented module. By increasing the entropy, the increased crystal symmetry delocalized the distribution of electrons in the distorted rhombohedral structure, resulting in band convergence and improved electrical properties. By contrast, the localized phonons from the entropy-induced disorder dampened the propagation of transverse phonons, which was the origin of the increased anharmonicity and largely depressed lattice thermal conductivity. We provide a paradigm for tuning electron and phonon localization by entropy manipulation, but we have also demonstrated a route for improving the performance of high-entropy thermoelectric materials.
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Jiang, B., Wang, W., Liu, S., Wang, Y., Wang, C., Chen, Y., Xie, L. H., Huang, M., & He, J. (2022). High figure-of-merit and power generation in high-entropy GeTe-based thermoelectrics. Science, 377(6602), 208–213. https://doi.org/10.1126/science.abq5815
Jiang, Binbin, et al. "High figure-of-merit and power generation in high-entropy GeTe-based thermoelectrics." Science, vol. 377, no. 6602, 2022, pp. 208–213, https://doi.org/10.1126/science.abq5815.
Jiang, Binbin, Wu Wang, Shixuan Liu, Yan Wang, Chaofan Wang, Yani Chen, Lin Hua Xie, Mingyuan Huang, and Jiaqing He. "High figure-of-merit and power generation in high-entropy GeTe-based thermoelectrics." Science 377, no. 6602 (2022): 208–213. https://doi.org/10.1126/science.abq5815.
Jiang B., Wang W., Liu S. [и др.] High figure-of-merit and power generation in high-entropy GeTe-based thermoelectrics // Science. — 2022. — Vol. 377, № 6602. — P. 208–213. — URL: https://doi.org/10.1126/science.abq5815
@article{jiang2022high,
title = {{High figure-of-merit and power generation in high-entropy GeTe-based thermoelectrics}},
author = {Binbin Jiang and Wu Wang and Shixuan Liu and Yan Wang and Chaofan Wang and Yani Chen and Lin Hua Xie and Mingyuan Huang and Jiaqing He},
journal = {Science},
year = {2022},
volume = {377},
number = {6602},
pages = {208--213},
doi = {10.1126/science.abq5815},
url = {https://doi.org/10.1126/science.abq5815}
}TY - JOUR AU - Jiang, Binbin AU - Wang, Wu AU - Liu, Shixuan AU - Wang, Yan AU - Wang, Chaofan AU - Chen, Yani AU - Xie, Lin Hua AU - Huang, Mingyuan AU - He, Jiaqing TI - High figure-of-merit and power generation in high-entropy GeTe-based thermoelectrics JO - Science VL - 377 IS - 6602 SP - 208 EP - 213 PY - 2022 DA - 2022/07/07 DO - 10.1126/science.abq5815 UR - https://doi.org/10.1126/science.abq5815 ER -
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