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Di Wang, Chenkun Zhou, Alexander S. Filatov, Wooje Cho, Francisco Lagunas, Mingzhan Wang, Suriyanarayanan Vaikuntanathan, Chong Liu, Robert F. Klie, Dmitri V. Talapin
Two-dimensional transition-metal carbides and nitrides (MXenes) are a large family of materials actively studied for various applications, especially in the field of energy storage. MXenes are commonly synthesized by etching the layered ternary compounds, called MAX phases. We demonstrate a direct synthetic route for scalable and atom-economic synthesis of MXenes, including compounds that have not been synthesized from MAX phases, by the reactions of metals and metal halides with graphite, methane, or nitrogen. The direct synthesis enables chemical vapor deposition growth of MXene carpets and complex spherulite-like morphologies that form through buckling and release of MXene carpet to expose fresh surface for further reaction. The directly synthesized MXenes showed excellent energy storage capacity for lithium-ion intercalation.
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Wang, D., Zhou, C., Filatov, A. S., Cho, W., Lagunas, F., Wang, M., Vaikuntanathan, S., Liu, C., Klie, R. F., & Talapin, D. V. (2023). Direct synthesis and chemical vapor deposition of 2D carbide and nitride MXenes. Science, 379(6638), 1242–1247. https://doi.org/10.1126/science.add9204
Wang, Di, et al. "Direct synthesis and chemical vapor deposition of 2D carbide and nitride MXenes." Science, vol. 379, no. 6638, 2023, pp. 1242–1247, https://doi.org/10.1126/science.add9204.
Wang, Di, Chenkun Zhou, Alexander S. Filatov, Wooje Cho, Francisco Lagunas, Mingzhan Wang, Suriyanarayanan Vaikuntanathan, Chong Liu, Robert F. Klie, and Dmitri V. Talapin. "Direct synthesis and chemical vapor deposition of 2D carbide and nitride MXenes." Science 379, no. 6638 (2023): 1242–1247. https://doi.org/10.1126/science.add9204.
Wang D., Zhou C., Filatov A. S. [и др.] Direct synthesis and chemical vapor deposition of 2D carbide and nitride MXenes // Science. — 2023. — Vol. 379, № 6638. — P. 1242–1247. — URL: https://doi.org/10.1126/science.add9204
@article{wang2023direct,
title = {{Direct synthesis and chemical vapor deposition of 2D carbide and nitride MXenes}},
author = {Di Wang and Chenkun Zhou and Alexander S. Filatov and Wooje Cho and Francisco Lagunas and Mingzhan Wang and Suriyanarayanan Vaikuntanathan and Chong Liu and Robert F. Klie and Dmitri V. Talapin},
journal = {Science},
year = {2023},
volume = {379},
number = {6638},
pages = {1242--1247},
doi = {10.1126/science.add9204},
url = {https://doi.org/10.1126/science.add9204}
}TY - JOUR AU - Wang, Di AU - Zhou, Chenkun AU - Filatov, Alexander S. AU - Cho, Wooje AU - Lagunas, Francisco AU - Wang, Mingzhan AU - Vaikuntanathan, Suriyanarayanan AU - Liu, Chong AU - Klie, Robert F. AU - Talapin, Dmitri V. TI - Direct synthesis and chemical vapor deposition of 2D carbide and nitride MXenes JO - Science VL - 379 IS - 6638 SP - 1242 EP - 1247 PY - 2023 DA - 2023/03/23 DO - 10.1126/science.add9204 UR - https://doi.org/10.1126/science.add9204 ER -
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