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Lina Chong, Guoping Gao, Jianguo Wen, Haixia Li, Haiping Xu, Zach Green, Joshua D. Sugar, Arthur Jeremy Kropf, Wenqian Xu, Xiao‐Min Lin and 3 more
Discovery of earth-abundant electrocatalysts to replace iridium for the oxygen evolution reaction (OER) in a proton exchange membrane water electrolyzer (PEMWE) represents a critical step in reducing the cost for green hydrogen production. We report a nanofibrous cobalt spinel catalyst codoped with lanthanum (La) and manganese (Mn) prepared from a zeolitic imidazolate framework embedded in electrospun polymer fiber. The catalyst demonstrated a low overpotential of 353 millivolts at 10 milliamperes per square centimeter and a low degradation for OER over 360 hours in acidic electrolyte. A PEMWE containing this catalyst at the anode demonstrated a current density of 2000 milliamperes per square centimeter at 2.47 volts (Nafion 115 membrane) or 4000 milliamperes per square centimeter at 3.00 volts (Nafion 212 membrane) and low degradation in an accelerated stress test.
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Chong, L., Gao, G., Wen, J., Li, H., Xu, H., Green, Z., Sugar, J. D., Kropf, A. J., Xu, W., Lin, X., Xu, H., Wang, L., & Liu, D. (2023). La- and Mn-doped cobalt spinel oxygen evolution catalyst for proton exchange membrane electrolysis. Science, 380(6645), 609–616. https://doi.org/10.1126/science.ade1499
Chong, Lina, et al. "La- and Mn-doped cobalt spinel oxygen evolution catalyst for proton exchange membrane electrolysis." Science, vol. 380, no. 6645, 2023, pp. 609–616, https://doi.org/10.1126/science.ade1499.
Chong, Lina, Guoping Gao, Jianguo Wen, Haixia Li, Haiping Xu, Zach Green, Joshua D. Sugar, et al. "La- and Mn-doped cobalt spinel oxygen evolution catalyst for proton exchange membrane electrolysis." Science 380, no. 6645 (2023): 609–616. https://doi.org/10.1126/science.ade1499.
Chong L., Gao G., Wen J. [и др.] La- and Mn-doped cobalt spinel oxygen evolution catalyst for proton exchange membrane electrolysis // Science. — 2023. — Vol. 380, № 6645. — P. 609–616. — URL: https://doi.org/10.1126/science.ade1499
@article{chong2023mndoped,
title = {{La- and Mn-doped cobalt spinel oxygen evolution catalyst for proton exchange membrane electrolysis}},
author = {Lina Chong and Guoping Gao and Jianguo Wen and Haixia Li and Haiping Xu and Zach Green and Joshua D. Sugar and Arthur Jeremy Kropf and Wenqian Xu and Xiao‐Min Lin and Hui Xu and Lin‐Wang Wang and Di‐Jia Liu},
journal = {Science},
year = {2023},
volume = {380},
number = {6645},
pages = {609--616},
doi = {10.1126/science.ade1499},
url = {https://doi.org/10.1126/science.ade1499}
}TY - JOUR AU - Chong, Lina AU - Gao, Guoping AU - Wen, Jianguo AU - Li, Haixia AU - Xu, Haiping AU - Green, Zach AU - Sugar, Joshua D. AU - Kropf, Arthur Jeremy AU - Xu, Wenqian AU - Lin, Xiao‐Min AU - Xu, Hui AU - Wang, Lin‐Wang AU - Liu, Di‐Jia TI - La- and Mn-doped cobalt spinel oxygen evolution catalyst for proton exchange membrane electrolysis JO - Science VL - 380 IS - 6645 SP - 609 EP - 616 PY - 2023 DA - 2023/05/11 DO - 10.1126/science.ade1499 UR - https://doi.org/10.1126/science.ade1499 ER -
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