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Zhen Li, Xianglang Sun, Xiaopeng Zheng, Bo Li, Danpeng Gao, Shoufeng Zhang, Xin Wu, Shuai Li, Jianqiu Gong, Joseph M. Luther, Zhong’an Li, Zonglong Zhu
P-i-n geometry perovskite solar cells (PSCs) offer simplified fabrication, greater amenability to charge extraction layers, and low-temperature processing over n-i-p counterparts. Self-assembled monolayers (SAMs) can enhance the performance of p-i-n PSCs but ultrathin SAMs can be thermally unstable. We report a thermally robust hole-selective layer comprised of nickel oxide (NiO x ) nanoparticle film with a surface-anchored (4-(3,11-dimethoxy-7H-dibenzo[c,g]carbazol-7-yl)butyl)phosphonic acid (MeO-4PADBC) SAM that can improve and stabilize the NiO x /perovskite interface. The energetic alignment and favorable contact and binding between NiO x /MeO-4PADBC and perovskite reduced the voltage deficit of PSCs with various perovskite compositions and led to strong interface toughening effects under thermal stress. The resulting 1.53–electron-volt devices achieved 25.6% certified power conversion efficiency and maintained >90% of their initial efficiency after continuously operating at 65 degrees Celsius for 1200 hours under 1-sun illumination.
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Li, Z., Sun, X., Zheng, X., Li, B., Gao, D., Zhang, S., Wu, X., Li, S., Gong, J., Luther, J. M., Li, Z., & Zhu, Z. (2023). Stabilized hole-selective layer for high-performance inverted p-i-n perovskite solar cells. Science, 382(6668), 284–289. https://doi.org/10.1126/science.ade9637
Li, Zhen, et al. "Stabilized hole-selective layer for high-performance inverted p-i-n perovskite solar cells." Science, vol. 382, no. 6668, 2023, pp. 284–289, https://doi.org/10.1126/science.ade9637.
Li, Zhen, Xianglang Sun, Xiaopeng Zheng, Bo Li, Danpeng Gao, Shoufeng Zhang, Xin Wu, et al. "Stabilized hole-selective layer for high-performance inverted p-i-n perovskite solar cells." Science 382, no. 6668 (2023): 284–289. https://doi.org/10.1126/science.ade9637.
Li Z., Sun X., Zheng X. [и др.] Stabilized hole-selective layer for high-performance inverted p-i-n perovskite solar cells // Science. — 2023. — Vol. 382, № 6668. — P. 284–289. — URL: https://doi.org/10.1126/science.ade9637
@article{li2023stabilized,
title = {{Stabilized hole-selective layer for high-performance inverted p-i-n perovskite solar cells}},
author = {Zhen Li and Xianglang Sun and Xiaopeng Zheng and Bo Li and Danpeng Gao and Shoufeng Zhang and Xin Wu and Shuai Li and Jianqiu Gong and Joseph M. Luther and Zhong’an Li and Zonglong Zhu},
journal = {Science},
year = {2023},
volume = {382},
number = {6668},
pages = {284--289},
doi = {10.1126/science.ade9637},
url = {https://doi.org/10.1126/science.ade9637}
}TY - JOUR AU - Li, Zhen AU - Sun, Xianglang AU - Zheng, Xiaopeng AU - Li, Bo AU - Gao, Danpeng AU - Zhang, Shoufeng AU - Wu, Xin AU - Li, Shuai AU - Gong, Jianqiu AU - Luther, Joseph M. AU - Li, Zhong’an AU - Zhu, Zonglong TI - Stabilized hole-selective layer for high-performance inverted p-i-n perovskite solar cells JO - Science VL - 382 IS - 6668 SP - 284 EP - 289 PY - 2023 DA - 2023/10/19 DO - 10.1126/science.ade9637 UR - https://doi.org/10.1126/science.ade9637 ER -
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