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Xianbiao Fu, Jakob Bruun Pedersen, Yuanyuan Zhou, Mattia Saccoccio, Shaofeng Li, Rokas Sažinas, Katja Li, Suzanne Zamany Andersen, Aoni Xu, Niklas H. Deissler and 6 more
Ammonia is a critical component in fertilizers, pharmaceuticals, and fine chemicals and is an ideal, carbon-free fuel. Recently, lithium-mediated nitrogen reduction has proven to be a promising route for electrochemical ammonia synthesis at ambient conditions. In this work, we report a continuous-flow electrolyzer equipped with 25-square centimeter-effective area gas diffusion electrodes wherein nitrogen reduction is coupled with hydrogen oxidation. We show that the classical catalyst platinum is not stable for hydrogen oxidation in the organic electrolyte, but a platinum-gold alloy lowers the anode potential and avoids the decremental decomposition of the organic electrolyte. At optimal operating conditions, we achieve, at 1 bar, a faradaic efficiency for ammonia production of up to 61 ± 1% and an energy efficiency of 13 ± 1% at a current density of -6 milliamperes per square centimeter.
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Fu, X., Pedersen, J. B., Zhou, Y., Saccoccio, M., Li, S., Sažinas, R., Li, K., Andersen, S. Z., Xu, A., Deissler, N. H., Mygind, J. B. V., Wei, C., Kibsgaard, J., Vesborg, P. C. K., Nørskov, J. K., & Chorkendorff, I. (2023). Continuous-flow electrosynthesis of ammonia by nitrogen reduction and hydrogen oxidation. Science, 379(6633), 707–712. https://doi.org/10.1126/science.adf4403
Fu, Xianbiao, et al. "Continuous-flow electrosynthesis of ammonia by nitrogen reduction and hydrogen oxidation." Science, vol. 379, no. 6633, 2023, pp. 707–712, https://doi.org/10.1126/science.adf4403.
Fu, Xianbiao, Jakob Bruun Pedersen, Yuanyuan Zhou, Mattia Saccoccio, Shaofeng Li, Rokas Sažinas, Katja Li, et al. "Continuous-flow electrosynthesis of ammonia by nitrogen reduction and hydrogen oxidation." Science 379, no. 6633 (2023): 707–712. https://doi.org/10.1126/science.adf4403.
Fu X., Pedersen J. B., Zhou Y. [и др.] Continuous-flow electrosynthesis of ammonia by nitrogen reduction and hydrogen oxidation // Science. — 2023. — Vol. 379, № 6633. — P. 707–712. — URL: https://doi.org/10.1126/science.adf4403
@article{fu2023continuousflow,
title = {{Continuous-flow electrosynthesis of ammonia by nitrogen reduction and hydrogen oxidation}},
author = {Xianbiao Fu and Jakob Bruun Pedersen and Yuanyuan Zhou and Mattia Saccoccio and Shaofeng Li and Rokas Sažinas and Katja Li and Suzanne Zamany Andersen and Aoni Xu and Niklas H. Deissler and Jon Bjarke Valbæk Mygind and Chao Wei and Jakob Kibsgaard and Peter C. K. Vesborg and Jens K. Nørskov and Ib Chorkendorff},
journal = {Science},
year = {2023},
volume = {379},
number = {6633},
pages = {707--712},
doi = {10.1126/science.adf4403},
url = {https://doi.org/10.1126/science.adf4403}
}TY - JOUR AU - Fu, Xianbiao AU - Pedersen, Jakob Bruun AU - Zhou, Yuanyuan AU - Saccoccio, Mattia AU - Li, Shaofeng AU - Sažinas, Rokas AU - Li, Katja AU - Andersen, Suzanne Zamany AU - Xu, Aoni AU - Deissler, Niklas H. AU - Mygind, Jon Bjarke Valbæk AU - Wei, Chao AU - Kibsgaard, Jakob AU - Vesborg, Peter C. K. AU - Nørskov, Jens K. AU - Chorkendorff, Ib TI - Continuous-flow electrosynthesis of ammonia by nitrogen reduction and hydrogen oxidation JO - Science VL - 379 IS - 6633 SP - 707 EP - 712 PY - 2023 DA - 2023/02/16 DO - 10.1126/science.adf4403 UR - https://doi.org/10.1126/science.adf4403 ER -
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