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Shuo Zhang, Fangyuan Ye, Xiaoyu Wang, Rui Chen, Huidong Zhang, Liqing Zhan, Xianyuan Jiang, Yawen Li, Xiaoyu Ji, Shuaijun Liu and 15 more
Controlling the perovskite morphology and defects at the buried perovskite-substrate interface is challenging for inverted perovskite solar cells. In this work, we report an amphiphilic molecular hole transporter, (2-(4-(bis(4-methoxyphenyl)amino)phenyl)-1-cyanovinyl)phosphonic acid, that features a multifunctional cyanovinyl phosphonic acid group and forms a superwetting underlayer for perovskite deposition, which enables high-quality perovskite films with minimized defects at the buried interface. The resulting perovskite film has a photoluminescence quantum yield of 17% and a Shockley-Read-Hall lifetime of nearly 7 microseconds and achieved a certified power conversion efficiency (PCE) of 25.4% with an open-circuit voltage of 1.21 volts and a fill factor of 84.7%. In addition, 1-square centimeter cells and 10-square centimeter minimodules show PCEs of 23.4 and 22.0%, respectively. Encapsulated modules exhibited high stability under both operational and damp heat test conditions.
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Zhang, S., Ye, F., Wang, X., Chen, R., Zhang, H., Zhan, L., Jiang, X., Li, Y., Ji, X., Liu, S., Yu, M., Yu, F., Zhang, Y., Wu, R., Liu, Z., Ning, Z., Neher, D., Han, L., Lin, Y., … Wu, Y. (2023). Minimizing buried interfacial defects for efficient inverted perovskite solar cells. Science, 380(6643), 404–409. https://doi.org/10.1126/science.adg3755
Zhang, Shuo, et al. "Minimizing buried interfacial defects for efficient inverted perovskite solar cells." Science, vol. 380, no. 6643, 2023, pp. 404–409, https://doi.org/10.1126/science.adg3755.
Zhang, Shuo, Fangyuan Ye, Xiaoyu Wang, Rui Chen, Huidong Zhang, Liqing Zhan, Xianyuan Jiang, et al. "Minimizing buried interfacial defects for efficient inverted perovskite solar cells." Science 380, no. 6643 (2023): 404–409. https://doi.org/10.1126/science.adg3755.
Zhang S., Ye F., Wang X. [и др.] Minimizing buried interfacial defects for efficient inverted perovskite solar cells // Science. — 2023. — Vol. 380, № 6643. — P. 404–409. — URL: https://doi.org/10.1126/science.adg3755
@article{zhang2023minimizing,
title = {{Minimizing buried interfacial defects for efficient inverted perovskite solar cells}},
author = {Shuo Zhang and Fangyuan Ye and Xiaoyu Wang and Rui Chen and Huidong Zhang and Liqing Zhan and Xianyuan Jiang and Yawen Li and Xiaoyu Ji and Shuaijun Liu and Miaojie Yu and Furong Yu and Yilin Zhang and Ruihan Wu and Zonghao Liu and Zhijun Ning and Dieter Neher and Liyuan Han and Yuze Lin and He Tian and Wei Chen and Martin Stolterfoht and Lijun Zhang and Weihong Zhu and Yongzhen Wu},
journal = {Science},
year = {2023},
volume = {380},
number = {6643},
pages = {404--409},
doi = {10.1126/science.adg3755},
url = {https://doi.org/10.1126/science.adg3755}
}TY - JOUR AU - Zhang, Shuo AU - Ye, Fangyuan AU - Wang, Xiaoyu AU - Chen, Rui AU - Zhang, Huidong AU - Zhan, Liqing AU - Jiang, Xianyuan AU - Li, Yawen AU - Ji, Xiaoyu AU - Liu, Shuaijun AU - Yu, Miaojie AU - Yu, Furong AU - Zhang, Yilin AU - Wu, Ruihan AU - Liu, Zonghao AU - Ning, Zhijun AU - Neher, Dieter AU - Han, Liyuan AU - Lin, Yuze AU - Tian, He AU - Chen, Wei AU - Stolterfoht, Martin AU - Zhang, Lijun AU - Zhu, Weihong AU - Wu, Yongzhen TI - Minimizing buried interfacial defects for efficient inverted perovskite solar cells JO - Science VL - 380 IS - 6643 SP - 404 EP - 409 PY - 2023 DA - 2023/04/27 DO - 10.1126/science.adg3755 UR - https://doi.org/10.1126/science.adg3755 ER -
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